PPPoE frames are just ethernet frames, and powerline adapters are just ethernet bridges, so it will work.
Using "baby jumbo frames" to your ONT (MTU 1508, so that you get an IP MTU of 1500) may or may not work.
But as others have said, powerline adapters are not really suitable at FTTP speeds. While they may have a "raw" bit rate of say 500Mbps, this is unidirectional, subject to contention, collisions, and noise. Real-world throughput is unlikely to be more than about a third of the headline figure.
For the best reliability, run a CAT5e cable from your ONT to your router.



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